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The recently demonstrated chiral modes of lattice motion carry angular momentum and therefore directly couple to magnetic fields. Notably, their magnetic moments are predicted to be strongly influenced by electronic contributions. Here, we have studied the magnetic response of transverse optical phonons in a set of Pb1−xSnxTe films, which is a topological crystalline insulator forx> 0.32 and has a ferroelectric transition at anx-dependent critical temperature. Polarization-dependent terahertz magnetospectroscopy measurements revealed Zeeman splittings and diamagnetic shifts, demonstrating a large phonon magnetic moment. Films in the topological phase exhibited phonon magnetic moment values that were larger than those in the topologically trivial samples by two orders of magnitude. Furthermore, the sign of the effective phonong-factor was opposite in the two phases, a signature of the topological transition according to our model. These results strongly indicate the existence of interplay between the magnetic properties of chiral phonons and the topology of the electronic band structure.more » « less
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Observation of colossal terahertz magnetoresistance and magnetocapacitance in a perovskite manganiteTerahertz (THz) magnetoresistance effects have been extensively investigated and have shown promising results for applications in magnetic modulations of the amplitude of THz waves. However, THz magnetocapacitance in dielectric systems, which is essential for phase modulations of THz radiation, remains largely unexplored. Here, we study the THz response of a bulk single crystal of La0.875Sr0.125MnO3at around its Curie temperature, observing significant magnetic-field-induced changes in the THz resistance and capacitance extracted from the optical conductivity. We discuss possible mechanisms for the observed coexistence of colossal THz magnetoresistance and magnetocapacitance in a perovskite manganite that is not multiferroic. This work enhances our understanding of colossal magnetoresistance in a complex system with THz spectroscopy and demonstrates potential use of perovskite manganites in THz technology.more » « less
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In terahertz (THz) photonics, there is an ongoing effort to develop thin, compact devices such as dielectric photonic crystal (PhC) slabs with desirable light–matter interactions. However, previous works in THz PhC slabs have been limited to rigid substrates with thicknesses of micrometers. Dielectric PhC slabs have been shown to possess in-plane modes that are excited by external radiation to produce sharp guided-mode resonances with minimal absorption for applications in sensors, optics, and lasers. Here we confirm the existence of guided resonances in a membrane-type THz PhC slab with subwavelength ( ) thicknesses of flexible dielectric polyimide films. The transmittance of the guided resonances was measured for different structural parameters of the unit cell. Furthermore, we exploited the flexibility of the samples to modulate the guided modes for a bend angle of , confirmed experimentally by the suppression of these modes. The mechanical flexibility of the device allows for an additional degree of freedom in system design for high-speed communications, soft wearable photonics, and implantable medical devices.more » « less
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Abstract Hybrid light–matter coupled states, or polaritons, in magnetic materials have attracted significant attention due to their potential for enabling novel applications in spintronics and quantum information processing. However, most magnon‐polariton studies in the strong coupling regime to date have been carried out for ferromagnetic materials with magnon excitations at gigahertz frequencies. Here, strong resonant photon–magnon coupling at frequencies above 1 terahertz is investigated for the first time in a prototypical room‐temperature antiferromagnetic insulator, NiO, inside a Fabry–Pérot cavity. The cavity is formed by the crystal itself with a thickness adjusted to an optimal value. Terahertz time‐domain spectroscopy measurements in magnetic fields up to 25 T reveal the evolution of the magnon frequency through Fabry–Pérot cavity modes with photon–magnon anticrossing behavior, demonstrating clear vacuum Rabi splittings exceeding the polariton linewidths. These results show that NiO is a promising platform for exploring antiferromagnetic spintronics and cavity magnonics in the terahertz frequency range.more » « less
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